I don't think it's possible because the group sum is a dynamically evaluated number per each group - and a sort only affects the individual rows.
An alternate route might be to do a project report where you use one of these fields (in your case I think it's Actual billable expense cost) and link to the project's billingRecords page?
These fields are also aggregates values but it's an actual value on the project so you would be able to sort on it.
